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Gauge invariance and Ward identities in nonlinear response theory
NORDITA SU.
Radboud Univ Nijmegen, Inst Mol & Mat, Heyendaalseweg 135, NL-6525 AJ Nijmegen, Netherlands..ORCID iD: 0000-0001-5165-7553
Univ Missouri, Dept Phys & Astron, Columbia, MO 65211 USA..
Univ Pisa, Dipartimento Fis, Largo Bruno Pontecorvo 3, I-56127 Pisa, Italy.;Ist Italiano Tecnol, Graphene Labs, Via Morego 30, I-16163 Genoa, Italy.;Univ Manchester, Sch Phys & Astron, Oxford Rd, Manchester M13 9PL, Lancs, England..
2021 (English)In: Annals of Physics, ISSN 0003-4916, E-ISSN 1096-035X, Vol. 431, article id 168523Article in journal (Refereed) Published
Abstract [en]

We present a formal analysis of nonlinear response functions in terms of correlation functions in real-and imaginary-time domains. In particular, we show that causal nonlinear response functions, expressed in terms of nested commutators in real time, can be obtained from the analytic continuation of time ordered response functions, which are more easily amenable to diagrammatic calculation. This generalizes the well-known result of linear response theory. We then use gauge invariance arguments to derive exact relations between second-order response functions in density and current channels. These identities, which are non-perturbative in the strength of inter-particle interactions, allow us to establish exact connections between nonlinear optics calculations done in different electromagnetic gauges.

Place, publisher, year, edition, pages
Elsevier BV , 2021. Vol. 431, article id 168523
Keywords [en]
Nonlinear optics, Gauge invariance, Ward identity
National Category
Subatomic Physics
Identifiers
URN: urn:nbn:se:kth:diva-303199DOI: 10.1016/j.aop.2021.168523ISI: 000696989200004Scopus ID: 2-s2.0-85108183312OAI: oai:DiVA.org:kth-303199DiVA, id: diva2:1601928
Note

Nordita SU, QC 20211011

Available from: 2021-10-11 Created: 2021-10-11 Last updated: 2022-06-25Bibliographically approved

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CiteExportLink to record
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