kth.sePublications KTH
Change search
CiteExportLink to record
Permanent link

Direct link
Cite
Citation style
  • apa
  • ieee
  • modern-language-association-8th-edition
  • vancouver
  • Other style
More styles
Language
  • de-DE
  • en-GB
  • en-US
  • fi-FI
  • nn-NO
  • nn-NB
  • sv-SE
  • Other locale
More languages
Output format
  • html
  • text
  • asciidoc
  • rtf
Following the Crystallization of Amorphous Ice after Ultrafast Laser Heating
Department of Physics, AlbaNova University Center, Stockholm University, Stockholm SE-10691, Sweden.ORCID iD: 0000-0003-1355-649x
Department of Physics, AlbaNova University Center, Stockholm University, Stockholm SE-10691, Sweden.ORCID iD: 0000-0002-7319-7807
Department of Chemistry, POSTECH, Pohang 37673, Republic of Korea.
Department of Physics, AlbaNova University Center, Stockholm University, Stockholm SE-10691, Sweden;SLAC National Accelerator Laboratory, 2575 Sand Hill Road, Menlo Park, California 94025, United States.
Show others and affiliations
2022 (English)In: Journal of Physical Chemistry B, ISSN 1520-6106, E-ISSN 1520-5207, Vol. 126, no 11, p. 2299-2307Article in journal (Refereed) Published
Abstract [en]

Using time-resolved wide-angle X-ray scattering, we investigated the early stages (10 μs–1 ms) of crystallization of supercooled water, obtained by the ultrafast heating of high- and low-density amorphous ice (HDA and LDA) up to a temperature T = 205 K ± 10 K. We have determined that the crystallizing phase is stacking disordered ice (Isd), with a maximum cubicity of χ = 0.6, in agreement with predictions from molecular dynamics simulations at similar temperatures. However, we note that a growing small portion of hexagonal ice (Ih) was also observed, suggesting that within our timeframe, Isd starts annealing into Ih. The onset of crystallization, in both amorphous ice, occurs at a similar temperature, but the observed final crystalline fraction in the LDA sample is considerably lower than that in the HDA sample. We attribute this discrepancy to the thickness difference between the two samples.

Place, publisher, year, edition, pages
American Chemical Society (ACS) , 2022. Vol. 126, no 11, p. 2299-2307
National Category
Atom and Molecular Physics and Optics
Identifiers
URN: urn:nbn:se:kth:diva-348975DOI: 10.1021/acs.jpcb.1c10906ISI: 000778011400016PubMedID: 35275642Scopus ID: 2-s2.0-85126546920OAI: oai:DiVA.org:kth-348975DiVA, id: diva2:1879084
Note

QC 20240701

Available from: 2024-06-27 Created: 2024-06-27 Last updated: 2024-07-01Bibliographically approved

Open Access in DiVA

No full text in DiVA

Other links

Publisher's full textPubMedScopus

Authority records

Ladd-Parada, Marjorie

Search in DiVA

By author/editor
Ladd-Parada, MarjorieAmann-Winkel, KatrinPerakis, FivosNilsson, Anders
In the same journal
Journal of Physical Chemistry B
Atom and Molecular Physics and Optics

Search outside of DiVA

GoogleGoogle Scholar

doi
pubmed
urn-nbn

Altmetric score

doi
pubmed
urn-nbn
Total: 53 hits
CiteExportLink to record
Permanent link

Direct link
Cite
Citation style
  • apa
  • ieee
  • modern-language-association-8th-edition
  • vancouver
  • Other style
More styles
Language
  • de-DE
  • en-GB
  • en-US
  • fi-FI
  • nn-NO
  • nn-NB
  • sv-SE
  • Other locale
More languages
Output format
  • html
  • text
  • asciidoc
  • rtf