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Magnetic structure and phase diagram of YbCo2; Specific heat, muon spin rotation and relaxation and neutron diffraction study
Institute of Physics, Czech Academy of Sciences, Na Slovance 2, Prague 8 182 21, Czech Republic; Charles University, Faculty of Mathematics and Physics, Department of Condensed Matter Physics, Prague 2 121 16, Czech Republic; Research Center for Materials Nanoarchitectonics (MANA), National Institute for Materials Science, 1-2-1, Sengen, Tsukuba, Ibaraki 305-0047, Japan.
Charles University, Faculty of Mathematics and Physics, Department of Condensed Matter Physics, Prague 2 121 16, Czech Republic.
Research Center for Materials Nanoarchitectonics (MANA), National Institute for Materials Science, 1-2-1, Sengen, Tsukuba, Ibaraki 305-0047, Japan.
Research Center for Materials Nanoarchitectonics (MANA), National Institute for Materials Science, 1-2-1, Sengen, Tsukuba, Ibaraki 305-0047, Japan.
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2025 (English)In: Journal of Alloys and Compounds, ISSN 0925-8388, E-ISSN 1873-4669, Vol. 1037, article id 182352Article in journal (Refereed) Published
Abstract [en]

This study explores the magnetic properties of YbCo2 through specific heat measurements, muon spin rotation spectroscopy, and neutron diffraction under external magnetic fields. A magnetic transition anomaly at 0.3 K in specific heat marks the onset of magnetic order, further corroborated by muon spin resonance data. A second anomaly in specific heat observed in an applied magnetic field indicates a field-induced change of magnetic ordering, confirmed by neutron diffraction experiment in magnetic fields. Yb magnetic moments exhibit a collinear ferromagnetic ordering, while Co moments align antiparallel to Yb moments at low magnetic fields. Increasing the external magnetic field, Co moments develop an additional antiferromagnetic component, modifying the overall magnetic structure. The observed magnetic order in low and high magnetic fields is consistently described by the single magnetic space group Imm'a’ and aligns well with theoretical predictions.

Place, publisher, year, edition, pages
Elsevier BV , 2025. Vol. 1037, article id 182352
Keywords [en]
Field-induced transitions, Intermetallics, Magnetic structure, Muon spin resonance, Neutron diffraction in magnetic fields, Phase diagram, Rare-earth RCo2, Specific heat, YbCo2
National Category
Condensed Matter Physics
Identifiers
URN: urn:nbn:se:kth:diva-368593DOI: 10.1016/j.jallcom.2025.182352ISI: 001542388000011Scopus ID: 2-s2.0-105011839478OAI: oai:DiVA.org:kth-368593DiVA, id: diva2:1989991
Note

QC 20250819

Available from: 2025-08-19 Created: 2025-08-19 Last updated: 2025-08-19Bibliographically approved

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Månsson, Martin

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